TY - EJOU AU - Kumar, Y. B. Kishore AU - Prasad, S. Guru AU - Smitha, A. S. Swapna AU - Chalapathi, U. AU - Babu, G. Suresh AU - Jayasree, Y. AU - Bhaskar, P. Uday AU - Park, Si-Hyun TI - Effect of carrier gas on copper antimony sulfide thin films by spray pyrolytic approach T2 - Chalcogenide Letters PY - 2024 VL - 21 IS - 9 SN - 1584-8663 AB - This study explores the ternary compound semiconductor as a potential absorber layer for third-generation solar cells. CuSbS2, a promising candidate for thin film absorber layers, is fabricated using a simple spray pyrolysis method. The research specifically investigates the influence of two different carrier gases during the fabrication process. X-ray diffraction as well as Raman studies confirm that the films exhibit a chalcostibite structure. Notably, films fabricated with nitrogen as the carrier gas demonstrate enhanced crystallinity, accompanied by reduced microstrain and dislocation density. Furthermore, these films exhibit a significantly improved absorption coefficient, reaching 105 cm-1 . Optical studies indicate that the materials possess a direct band gap of 1.50 eV and exhibit p-type conductivity. CuSbS2 thin film heterojunction solar cell exhibits a maximum efficiency of 0.49%. KW - CuSbS2 KW - Thin films KW - Spray pyrolytic technique KW - Carrier gases KW - Solar cell DO -