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g-C3N4 Derived Materials for Photocatalytic Hydrogen Production: A Mini Review on Design Strategies

Kai Su1,*, Shaoqi Deng1, Linxiao Li1, Qirui Qin1, Jingyu Yang1, Yan Chen2,3, Shengli Zhang1, Junming Chen1

1 Faculty of Geosciences and Environmental Engineering, Southwest Jiaotong University, Chengdu, 611756, China
2 Analysis and Testing Center, South China Normal University, Guangzhou, 510006, China
3 MOE Key Laboratory of Theoretical Chemistry of the Environment, School of Chemistry, South China Normal University, Guangzhou, 510006, China

* Corresponding Author: Kai Su. Email: email

Journal of Renewable Materials 2022, 10(3), 653-663. https://doi.org/10.32604/jrm.2022.018556

Abstract

Hydrogen production through solar energy is one of the most important pathways to meet the growing demand of renewable energy, and photocatalyst participation in solar hydrolytic hydrogen production has received great attention in recent years in terms of low cost, high efficiency, and flexible design. Particularly, g-C3N4 (Graphitic-like carbon nitride material), as a unique material, can catalyze the hydrogen production process by completing the separation and transmission of charge. The easily adjustable pore structure/surface area, dimension, band-gap modulation and defect have shown great potential for hydrogen production from water cracking. In this review, the most recent advance of g-C3N4 including the doping of metal and non-metal elements, and the formation of semiconductor heterojunction is highlighted. The main modification strategies and approaches for the design of g-C3N4 for hydrogen production, as well as the influence of various materials on hydrogen evolution regarding the photocatalysis mechanism and advantages brought by theoretical calculations are specially and briefly illustrated. Potential design pathways and strategies of g-C3N4 are discussed. In addition, current challenges of hydrogen production from g-C3N4 water splitting are summarized and can be expected.

Graphical Abstract

g-C<sub>3</sub>N<sub>4</sub> Derived Materials for Photocatalytic Hydrogen Production: A Mini Review on Design Strategies

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Cite This Article

Su, K., Deng, S., Li, L., Qin, Q., Yang, J. et al. (2022). g-C3N4 Derived Materials for Photocatalytic Hydrogen Production: A Mini Review on Design Strategies. Journal of Renewable Materials, 10(3), 653–663.

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cc This work is licensed under a Creative Commons Attribution 4.0 International License , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
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