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  • Open Access

    REVIEW

    Plant-Based Cellulose Nanopapers with Applications for Packaging, Protective Films and Energy Devices

    Verónica L. Mucci, Mirta I. Aranguren*

    Journal of Renewable Materials, Vol.13, No.8, pp. 1491-1519, 2025, DOI:10.32604/jrm.2025.02024-0079 - 22 August 2025

    Abstract Interest in the use of cellulose nanomaterial’s continues to grow, both in research and industry, not only due to the abundance of raw materials, low toxicity and sustainability, but also due to the attractive physical and chemical properties that make nanocelluloses useful for a wide range of end-use applications. Among the large number of potential uses, and nanocelluloses modification and processing strategies, the chosen topic of this review focuses exclusively on plant-derived cellulose microfibers/nanofibers (CNF) and cellulose nanocrystals (CNC) processed into 2D structures—nanopapers and nanofilms—fabricated as self-standing films or applied as coatings. The end uses… More > Graphic Abstract

    Plant-Based Cellulose Nanopapers with Applications for Packaging, Protective Films and Energy Devices

  • Open Access

    REVIEW

    Nanocellulose-Based Adhesives for Sustainable Wood-Polymer Composites: Recent Advancement and Future Perspective

    Amelia Hariry1, Efri Mardawati1,2,*, Apri Heri Iswanto3, Tati Karliati4, Lukmanul Hakim Zaini5,6,*, Muhammad Adly Rahandi Lubis2,7

    Journal of Renewable Materials, Vol.13, No.4, pp. 773-798, 2025, DOI:10.32604/jrm.2025.058359 - 21 April 2025

    Abstract Nanocellulose-based adhesives are gaining attention as a viable alternative to conventional adhesives, offering benefits such as cost-effectiveness and scalability, which make them suitable for various sectors, including cosmetics, pharmaceuticals, biodegradable products, and as reinforcing agents in natural adhesives. This review delves into the current advancements in nanocellulose-based adhesive solutions for sustainable and eco-friendly wood composites, using systematic review methods and bibliometric analysis. Data were collected from the Scopus database, spanning from 2007 to 2024, and visualized using VOSviewer to highlight emerging trends in the field. The analysis revealed that nanocellulose shows great potential as a More >

  • Open Access

    ARTICLE

    Effect of Mixing Strategy on the Structure-Properties of the PLA/PBAT Blends Incorporated with CNC

    Deniz Sema Sarul1, Dogan Arslan2, Emre Vatansever1, Yusuf Kahraman2, Ali Durmus3, Reza Salehiyan4, Mohammadreza Nofar1,2,*

    Journal of Renewable Materials, Vol.10, No.1, pp. 149-164, 2022, DOI:10.32604/jrm.2022.017003 - 27 July 2021

    Abstract Polylactide (PLA)/poly (butylene adipate-co-terephthalate) (PBAT) blend nanocomposites including 3 wt% of cellulose nanocrystals (CNCs) were prepared by melt compounding method in a twin-screw extruder and an internal mixer. Blend nanocomposites were formulated by diluting three different masterbatches prepared by solution casting method that contained 7 wt% of CNC. These masterbatches were: (m1) PLA/PBAT/CNC masterbatch; (m2) PLA/CNC masterbatch; and (m3) PBAT/CNC masterbatch. These were to explore how different preparation methods affect the dispersion and localization of CNC and hence the properties of PLA/PBAT/CNC blend nanocomposites. Scanning electron microscopy (SEM) was used to study the structural changes… More >

  • Open Access

    ARTICLE

    The Application of Cellulose Nanocrystals Modified with Succinic Anhydride under the Microwave Irradiation for Preparation of Polylactic Acid Nanocomposites

    Ewa Szefer*, Agnieszka Leszczyńska, Edyta Hebda, Krzysztof Pielichowski

    Journal of Renewable Materials, Vol.9, No.6, pp. 1127-1142, 2021, DOI:10.32604/jrm.2021.014584 - 11 March 2021

    Abstract The aim of this work was to use cellulose nanocrystals that were obtained by hydrolysis in phosphoric acid solution and further modified with succinic anhydride in the microwave field for PLA reinforcement. A series of all-bionanocomposites containing unmodified and surface modified cellulose nanocrystals with CNC content in the range of 1–3 %w.t. were obtained by melt blending and tested by XRD, SEM, DSC and DMA to investigate the effect of surface esterification of CNCs on the structure, morphology, dynamic mechanical properties of bionanocomposites, as well as phase transitions of PLA in the presence of cellulosic nanofiller. More > Graphic Abstract

    The Application of Cellulose Nanocrystals Modified with Succinic Anhydride under the Microwave Irradiation for Preparation of Polylactic Acid Nanocomposites

  • Open Access

    ARTICLE

    Preparation of Dicarboxyl Cellulose Nanocrystals from Agricultural Wastes by Sequential Periodate-Chlorite Oxidation

    Xiaozheng Sun*, Qiang He, Yu Yang

    Journal of Renewable Materials, Vol.8, No.4, pp. 447-460, 2020, DOI:10.32604/jrm.2020.09671 - 24 April 2020

    Abstract Agricultural waste straw is the renewable resource with the highest annual yield in the world. In value-added applications of agricultural waste, dicarboxyl cellulose nanocrystals (DCCs) are prepared from rice, wheat, and corn straw by sequential periodate-chlorite oxidation. In this study, DCCs from rice, wheat, and corn straw were characterized by transmission electron microscopy (TEM), Fourier transform infrared spectrometer, X-ray diffractometer (XRD), and thermal gravimetric analysis (TGA). The carboxyl content of the DCCs was also investigated. XRD results show that the crystallinity index decreased after sequential periodate-chlorite oxidation; however, the cellulose I structure was maintained. TEM… More >

  • Open Access

    ARTICLE

    Composite Biomaterials Based on Poly(L-Lactic Acid) and Functionalized Cellulose Nanocrystals

    Mariia Stepanova1, Ilia Averianov1, Olga Solomakha1, Natalia Zabolotnykh2, Iosif Gofman1, Mikhail Serdobintsev2, Tatiana Vinogradova2, Viktor Korzhikov-Vlakh1,3, Evgenia Korzhikova-Vlakh1,3,*

    Journal of Renewable Materials, Vol.8, No.4, pp. 383-395, 2020, DOI:10.32604/jrm.2020.09206 - 24 April 2020

    Abstract The biocomposite films were prepared from poly(L-lactic acid) and cellulose nanocrystals. To improve interfacial compatibility of hydrophilic cellulose nanocrystals with hydrophobic matrix polymer as well as to provide the osteoconductive properties, cellulose was functionalized with poly(glutamic acid). The modified cellulose nanocrystals were better distributed and less aggregated within the matrix, which was testified by scanning electron, optical and polarized light microscopy. According to mechanical tests, composites filled with nanocrystals modified with PGlu demonstrated higher values of Young’s modulus, elongation at break and tensile strength. Incubation of composite materials in model buffer solutions for 30 weeks More >

  • Open Access

    ARTICLE

    Isolation of Thermally Stable Cellulose Nanocrystals from Spent Coffee Grounds via Phosphoric Acid Hydrolysis

    Brody A. Frost, E. Johan Foster*

    Journal of Renewable Materials, Vol.8, No.2, pp. 187-203, 2020, DOI:10.32604/jrm.2020.07940 - 01 February 2020

    Abstract As the world's population exponentially grows, so does the need for the production of food, with cereal production growing annually from an estimated 1.0 billion to 2.5 billion tons within the last few decades. This rapid growth in food production results in an ever increasing amount of agricultural wastes, of which already occupies nearly 50% of the total landfill area. For example, is the billions of dry tons of cellulose-containing spent coffee grounds disposed in landfills annually. This paper seeks to provide a method for isolating cellulose nanocrystals (CNCs) from spent coffee grounds, in order… More >

  • Open Access

    ARTICLE

    Adsorption Behavior of Reducing End-Modified Cellulose Nanocrystals: A Kinetic Study Using Quartz Crystal Microbalance

    Maud Chemin, Céline Moreau, Bernard Cathala, Ana Villares*

    Journal of Renewable Materials, Vol.8, No.1, pp. 29-43, 2020, DOI:10.32604/jrm.2020.07850 - 01 January 2020

    Abstract In this work, we studied the adsorption of modified cellulose nanocrystals onto solid surfaces by quartz crystal microbalance with dissipation monitoring (QCM-D). Cellulose nanocrystals obtained from tunicate (CNC) were modified at reducing end by amidation reactions. Two different functionalities were investigated: a polyamine dendrimer (CNC-NH2), which interacts with gold surface by the amine groups; and a biotin moiety (CNC-Biot), which has a strong affinity for the protein streptavidin (SAV). QCM-D results revealed different adsorption behaviors between modified and unmodified CNCs. Hence, unmodified CNCs covered almost all the surface forming a rigid and flat layer whereas reducing More >

  • Open Access

    ARTICLE

    Influence of Xyloglucan Molar Mass on Rheological Properties of Cellulose Nanocrystal/Xyloglucan Hydrogels

    Malika Talantikite1,*, Antoine Gourlay1, Sophie Le Gall1, Bernard Cathala1

    Journal of Renewable Materials, Vol.7, No.12, pp. 1381-1390, 2019, DOI:10.32604/jrm.2019.07838

    Abstract Plant components are an inexhaustible source for the construction of bio-based materials. Here we report, for the first time, the elaboration of biobased cellulose nanocrystals (CNC)/xyloglucan (XG) hydrogels. XG is a hemicellulose displaying a great affinity for cellulose surface and can be thus irreversibly adsorbed on CNC. Properties of the hydrogels were investigated by varying the molar mass of XG either by enzymatic treatment with Endoglucanase (EG2) or physical fractionation by ultrasound (US). Fractions were characterised by high-performance size exclusion chromatography (HPSEC) and their monosacchari decompositions were determined. Three fractions with high, average and small… More >

  • Open Access

    ARTICLE

    Poly (Butylene Adipate-Co-Terephthalate) and Poly (Ɛ-Caprolactone) and Their Bionanocomposites with Cellulose Nanocrystals: Thermo-Mechanical Properties and Cell Viability Study

    Marcia Cristina Branciforti1,*, Caroline Faria Bellani2, Carolina Lipparelli Morelli2, Alice Ferrand3, Nadia Benkirane-Jessel3, Rosario Elida Suman Bretas2

    Journal of Renewable Materials, Vol.7, No.3, pp. 269-277, 2019, DOI:10.32604/jrm.2019.01833

    Abstract Although nanocomposites have recently attracted special interest in the tissue engineering area, due to their potential to reinforce scaffolds for hard tissues applications, a number of variables must be set prior to any clinical application. This manuscript addresses the evaluation of thermo-mechanical properties and of cell proliferation of cellulose nanocrystals (CNC), poly(butylene adipate-co-terephthalate) (PBAT), poly(ε-caprolactone) (PCL) films and their bionanocomposites with 2 wt% of CNC obtained by casting technique. Cellulose nanocrystals extracted from Balsa wood by acid hydrolysis were used as a reinforcing phase in PBAT and PCL matrix films. The films and pure CNC… More >

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