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  • Open Access

    ARTICLE

    Biobenzoxazines Generated in Hardened Tannin-Hexamine Wood Adhesives

    Antonio Pizzi*

    Journal of Renewable Materials, Vol.14, No.7, 2026, DOI:10.32604/jrm.2026.02026-0056 - 28 July 2026

    Abstract Cross Polarization Magic Angle Spinning Carbon 13 Nuclear Magnetic Resonance (CP-MAS 13C NMR) analysis of commercial procyanidin (pine bark) and delphinidin (pecan nut membranes) condensed flavonoid tannin extracts reacted with hexamethylenetetramine (hexamine) have shown that due to the highly reactive imino-amino methylene species formed before its degradation reaches the generation of formaldehyde, benzylamine bridges between the flavonoid units are formed. This study shows that tannin-based biobenzoxazines are also generated at the same time, with both benzylamines and benzoxazines bridges being in more marked proportions, the more reactive the tannin reacted with hexamethylenetetramine is. This is not More > Graphic Abstract

    Biobenzoxazines Generated in Hardened Tannin-Hexamine Wood Adhesives

  • Open Access

    ARTICLE

    Sustainable Particleboards Using Lignosulfonate-Modified MUF Adhesives for Enhanced Bond Strength and Reduced Formaldehyde Emissions

    Pavlo Bekhta1,2,*, Iryna Lytvyn1

    Journal of Renewable Materials, Vol.14, No.5, 2026, DOI:10.32604/jrm.2026.02026-0035 - 28 May 2026

    Abstract The modification of melamine–urea–formaldehyde (MUF) adhesives with lignosulfonates (LS) represents a promising strategy for developing more sustainable wood-based panels. However, the influence of the counterion type remains poorly understood. In this study, the effect of lignosulfonate counterions on adhesives performance and properties of MUF-bonded particleboards was investigated, with a focus on sodium (NaLS) and magnesium (MgLS) lignosulfonates incorporated at 2.5%, 5.0%, and 7.5%. Adhesives performance was characterized by measuring dry solids content, dynamic viscosity, gelation time, and pH. The produced particleboards were evaluated in terms of density, bending strength, modulus of elasticity, internal bond strength… More > Graphic Abstract

    Sustainable Particleboards Using Lignosulfonate-Modified MUF Adhesives for Enhanced Bond Strength and Reduced Formaldehyde Emissions

  • Open Access

    ARTICLE

    Maleated Deep Eutectic Solvent (DES) Lignin-Glyoxal-Chitosan Wood Adhesives

    Hamed Younesi-Kordkheili1,*, Antonio Pizzi2,*, Ghorban Niyatzadeh3

    Journal of Renewable Materials, Vol.14, No.4, 2026, DOI:10.32604/jrm.2026.02026-0013 - 24 April 2026

    Abstract In this research, an effective method has been developed to bond wood panel adhesives of good performance using biosourced lignin and chitosan as the two main raw materials. Lignin was thus modified by a deep eutectic solvent (DES) and maleic anhydride (MA), respectively. Then DES/MA modified lignin was reacted with glyoxal to obtain a new environmentally friendly lignin-glyoxal (LG) resin. Next, chitosan was added as a bio-crosslinker to the synthesised LG resin. Finally, the performance of the resulting adhesives was evaluated by bonding plywood panels with them. Fourier Transform Infra Red (FTIR) analysis was used… More > Graphic Abstract

    Maleated Deep Eutectic Solvent (DES) Lignin-Glyoxal-Chitosan Wood Adhesives

  • Open Access

    ARTICLE

    Citric Acid as an Alternative Adhesive: Optimisation of Concentrations on Characteristics of Jabon Plywood

    Muhammad Ilham Aulia1, Alifah Syahfitri1, Imam Busyra Abdillah1, Abdus Syukur1, Dede Hermawan1,*, Rita Kartika Sari1, Mahdi Mubarok1, Muhammad Adly Rahandi Lubis2, Sukma Surya Kusumah2, Sarah Augustina2, Jajang Sutiawan2,*

    Journal of Renewable Materials, Vol.14, No.4, 2026, DOI:10.32604/jrm.2025.02025-0160 - 24 April 2026

    Abstract Citric acid adhesive is an alternative to formaldehyde-based adhesives that are more environmentally friendly because they are non-toxic and made from natural ingredients. This study aims to determine the effect of variations in citric acid adhesive concentrations on the physical and mechanical properties of jabon plywood. This study used citric acid adhesive with variations in citric acid (CA) concentrations of 59%, 69%, and 79%. Physical property tests include density, moisture content (MC), water absorption (WA), thickness expansion (TS), and delamination, while mechanical tests include modulus of rupture (MOR), modulus of elasticity (MOE), and shear stress… More >

  • Open Access

    ARTICLE

    Numerical Determination of Weak Adhesive Bonds Using Ultrasonic Guided Waves

    Egidijus Žukauskas1,*, Damira Smagulova1, Elena Jasiūnienė1,2

    CMES-Computer Modeling in Engineering & Sciences, Vol.146, No.3, 2026, DOI:10.32604/cmes.2026.077492 - 30 March 2026

    Abstract Adhesively bonded joints are widely used in modern lightweight structures due to their high strength-to-weight ratio and design flexibility. However, the reliable non-destructive evaluation of bond integrity remains a significant challenge. This study presents a numerical investigation of adhesively bonded joints with different adhesive properties using ultrasonic guided waves. The main focus of the investigation is to evaluate the feasibility of using guided waves to assess bond integrity, particularly for detecting challenging weak bonds. For this purpose, a theoretical analysis of dispersion curves was conducted, revealing that the S0 Lamb wave mode is significantly sensitive… More >

  • Open Access

    ARTICLE

    Potential of Quebracho Tannin to Substitute Urea-Formaldehyde Adhesive in Plywood: Comparative Technical and Environmental Performance

    Belén Rovira1,*, Aude Chabrelie1, Sauro Bianchi2, Frédéric Pichelin1

    Journal of Renewable Materials, Vol.14, No.3, 2026, DOI:10.32604/jrm.2025.02025-0173 - 25 March 2026

    Abstract The construction sector is facing significant challenges in transitioning to a defossilised system. While wood-based products have considerable potential, reliance on adhesives derived from fossil fuels poses significant sustainability concerns. Tannin-based adhesives present a compelling bio-based alternative, offering advantageous bonding properties with the potential to reduce toxicity, minimise fossil resource use, and enhance end-of-life scenarios. Despite extensive research demonstrating the technical potential of tannin-based adhesives, industrial adoption remains limited—partly due to the paucity of studies addressing their environmental impacts. The present study investigates the use of tannin-based adhesives in the production of interior-grade plywood, employing… More >

  • Open Access

    ARTICLE

    Sustainable Particleboards Based on Sugarcane Bagasse and Bonded with a Waste-Grown Black Soldier Fly Larvae Commercial Flour-Based Adhesive: Rheological, Physical, and Mechanical Properties

    Francisco Daniel García1,2, Solange Nicole Aigner1,2, Natalia Raffaeli3, Antonio José Barotto3, Eleana Spavento3, Mariano Martín Escobar1,4, Marcela Angela Mansilla1,4, Alejandro Bacigalupe1,4,*

    Journal of Renewable Materials, Vol.14, No.1, 2026, DOI:10.32604/jrm.2025.02025-0181 - 23 January 2026

    Abstract This study explores the use of black soldier fly larvae protein as a bio-based adhesive to produce particleboards from sugarcane bagasse. A comprehensive evaluation was conducted, including rheological characterization of the adhesive and physical–mechanical testing of the panels according to European standards. The black soldier fly larvae-based adhesive exhibited gel-like viscoelastic behavior, rapid partial structural recovery after shear, and favorable application properties. Particleboards manufactured with this adhesive and sugarcane bagasse achieved promising mechanical performance, with modulus of rupture and modulus of elasticity values of 30.2 and 3500 MPa, respectively. Internal bond strength exceeded 0.4 MPa,… More > Graphic Abstract

    Sustainable Particleboards Based on Sugarcane Bagasse and Bonded with a Waste-Grown Black Soldier Fly Larvae Commercial Flour-Based Adhesive: Rheological, Physical, and Mechanical Properties

  • Open Access

    ARTICLE

    Plywood Bio-Adhesives by Oxidized Lignin Urea Bridged with Oxidized Starch

    Hamed Younesi-Kordkheili1,*, Antonio Pizzi2,*

    Journal of Renewable Materials, Vol.14, No.1, 2026, DOI:10.32604/jrm.2025.02025-0179 - 23 January 2026

    Abstract The aim of this research was to synthesize a new totally bio wood adhesive entailing the use of oxidized starch (OST), urea, and oxidized lignin (OL). For this reason, non-modified (L) and oxidized lignin (OL) at different contents (20%, 30%, and 40%) were used to prepare the starch-urea-lignin (SUL) and starch-urea-oxidized lignin (SUOL) resin. Sodium persulfate (SPS) as oxidizer was employed to oxidize both starch and lignin. Urea was just used as a low cost and effective crosslinker in the resin composition. The properties of the synthesized resins and the plywood panels bonded with them… More > Graphic Abstract

    Plywood Bio-Adhesives by Oxidized Lignin Urea Bridged with Oxidized Starch

  • Open Access

    ARTICLE

    Molasses Adhesive Boosts Bio-Pellet Potential: A Study on Oyster Mushroom Baglog Waste

    Sarah Augustina1, Ananda Suci Bazhafah2, Jajang Sutiawan1, Sudarmanto1, Eko Setio Wibowo1, Nissa Nurfajrin Solihat1, Alvin Muhammad Savero1, Ismadi Ismadi1, Jayadi Jayadi3, Agus Sukarto Wismogroho4, Nuniek Ina Ratnaningtyas2, Sukma Surya Kusumah1,*

    Journal of Renewable Materials, Vol.13, No.9, pp. 1765-1781, 2025, DOI:10.32604/jrm.2025.02025-0014 - 22 September 2025

    Abstract The increasing demand for renewable energy sources has driven the exploration of innovative materials for biofuel production. This study investigates bio-pellet characteristics derived from several oyster mushroom baglog wastes with varying concentrations of molasses as an adhesive. The process began with sun-drying the baglog waste for three days, followed by oven drying at 80°C for 24 h. Bio-pellets were produced by blending baglog waste with molasses at concentrations of 5% and 10% (w/v), then subsequently fed into a pellet mill. The bio-pellets were left to rest for one hour before analysis. The quality of bio-pellets… More > Graphic Abstract

    Molasses Adhesive Boosts Bio-Pellet Potential: A Study on Oyster Mushroom Baglog Waste

  • Open Access

    ARTICLE

    Eco-Friendly Particleboards Produced with Banana Tree (Musa paradisiaca) Pseudostem Fibers Bonded with Cassava Starch and Urea-Formaldehyde Adhesives

    Prosper Mensah1, Rafael Rodolfo de Melo2, Edgley Alves de Oliveira Paula2, Alexandre Santos Pimenta3, Juliana de Moura2, Fernando Rusch2,*

    Journal of Renewable Materials, Vol.13, No.7, pp. 1475-1489, 2025, DOI:10.32604/jrm.2025.02025-0047 - 22 July 2025

    Abstract The increase in wood and wood-based products in the construction and furniture sectors has grown exponentially, generating severe environmental and socioeconomic impacts. Particleboard panels have been the main cost-benefit option on the market due to their lightness and lower cost compared to solid wood. However, the synthetic adhesives used in producing traditional particleboard panels cause serious harm to human health. Developing particleboard panels with fibrous waste and natural adhesives could be a sustainable alternative for these sectors. The work aimed to create particleboards with fibrous wastes from the pseudostem of the banana tree (Musa paradisiaca) and… More > Graphic Abstract

    Eco-Friendly Particleboards Produced with Banana Tree (<i>Musa paradisiaca</i>) Pseudostem Fibers Bonded with Cassava Starch and Urea-Formaldehyde Adhesives

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